中国科学院高能物理研究所核能放射化学实验室---

: 袁立永
: 电子邮箱：yuanly@ihep.ac.cn

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袁立永，研究员。2015年获高能物理研究所“优秀青年人才基金”；2017年入选中国科学院青年创新促进会；2019年被遴选为中国化学会铀元素代言人。

教育及工作经历：
2021.9-至今在中国科学院高能物理研究所工作，研究员
2019.4-2021.8 在中国科学院高能物理研究所工作，特聘青年研究员
2012.8-2019.3 在中国科学院高能物理研究所工作，副研究员
2010.7-2012.7 在中国科学院高能物理研究所工作，助理研究员
2005.9-2010.7 在北京大学化学与分子工程学院应用化学专业硕博连读，获理学博士学位
2001.9-2005.7 在中国矿业大学化工学院应用化学专业读本科，获理学学士学位

研究方向：
1. 放化分离材料与技术；
2. 锕系离子的液液萃取分离与机理；
3. 同步辐射技术等核技术手段在锕系环境放射化学中的应用；

主持项目情况：
1. 基金委面上项目，2018.1～2021.12，金属有机骨架（MOF）材料在铀、钍吸附分离中的构效关系研究。项目资助金额65万。
2. 基金委面上项目，2015.1～2018.12，锕系组分离多官能团化介孔材料的设计制备及其辐射稳定性研究。项目资助金额85万。
3. 基金委-中国科学院大科学装置联合基金项目，2015.1～2017.12，功能化磁性纳米复合材料的设计制备及其对锕离子的吸附与分离研究。项目资助金额66 万。

代表性论文：

1. Pengliang Liang, Liyong Yuan*, Ke Du, Lin Wang, Zijie Li , Hao Deng, Xucong Wang, Shi-zhong Luo*, and Weiqun Shi*. Photocatalytic Reduction of Uranium(VI) under Visible Light with 2D/1D Ti3C2/CdS.

Chem. Eng. J. 2021, 420, 129831.

2. Bin Zhao, Liyong Yuan*, Yue Wang, Tao Duan*, Weiqun Shi*. Carboxylated UiO-66 Tailored for U(VI) and Eu(III) Trapping: from Batch Adsorption to Dynamic Column Separation.

ACS Appl. Mater. Interfaces 2021, 13, 16300-16308.

3. Ji-Pan Yu, JianHui Lan, Shuai Wang, Peng-Cheng Zhang, Kang Liu, Li-Yong Yuan*, Zhi-Fang Chai and Wei-Qun Shi*. Robust covalent organic frameworks with tailor-made chelating sites for synergistic capture of U(VI) ions from highly acidic radioactive waste.

Dalton Trans. 2021, 50, 3792-3796. (The first two authors contributed equally to this work)

4. Peng Ren, Pin-Wen Huang, Xiao-Fan Yang, Yao Zou, Wu-Qing Tao, Su-Liang Yang, Qun-Yan Wu, Li-Yong Yuan*, Zhi-Fang Chai and Wei-Qun Shi*. Hydrophilic Sulfonated 2,9-Diamide-1,10-Phenanthroline Endowed with Highly Effective Ligand for Separation Americium(III) from Europium(III): Extraction, Spectroscopy, and DFT Calculations.

Inorg. Chem. 2021, 60, 1, 357–365.

5. Yue Wang, Mingshu Xie, Jianhui Lan, Li-Yong Yuan*, Jipan Yu, Jiuqiang Li, Jing Peng, Zhifang Chai, John K. Gibson, Maolin Zhai* and Weiqun Shi*. Radiation controllable synthesis of robust covalent organic framework conjugates for efficient dynamic column extraction of 99TcO4−.

Chem. 2020, 6, 2796-2809.

6. Peng Ren, Cong-Zhi Wang, Wu-Qing Tao, Xiao-Fan Yang, Su-Liang Yang, Li-Yong Yuan*, Zhi-Fang Chai and Wei-Qun Shi*. Selective Separation and Coordination of Europium(III) and Americium(III) by Bisdiglycolamide: Solvent Extraction, Spectroscopy and DFT Calculations.

Inorg. Chem. 2020, 59, 14218–14228. (The first two authors contributed equally to this work).

7. Zhi-Hui Zhang, Jian-Hui Lan, Li-Yong Yuan*, Pan-Pan Sheng, Ming-Yang He, Li-Rong Zheng, Qun Chen, Zhi-Fang Chai, John K. Gibson and Wei-Qun Shi*. Rational Construction of Porous Metal–Organic Frameworks for Uranium(VI) Extraction: The Strong Periodic Tendency with a Metal Node.

ACS Appl. Mater. Interfaces 2020, 12(12), 14087-14094.

8. Lin Wang, Zi-Jie Li, Qun-Yan Wu, Zhi-Wei Huang, Li-YongYuan*, Zhi-Fang Chai and Wei-Qun Shi*. Layered structure-based materials: challenges and opportunities for radionuclide sequestration.

Environ. Sci.: Nano. 2020, 7: 724-752.

9. Peng-Liang Liang, Li-Yong Yuan*, Hao Deng, Xu-Cong Wang, Lin Wang, Zi-Jie Li, Shi-Zhong Luo* and Wei-Qun Shi*. Photocatalytic reduction of uranium(VI) by magnetic ZnFe2O4 under visible light.

Appl. Catal. B: Environ. 2020, 267, 118688.

10. Li-Yong Yuan, Ge Gao, Chuan-Qi Feng, Zhi-Fang Chai and Wei-Qun Shi*. A new family of actinide sorbents with more open porous structure: Fibrous functionalized silica microspheres.

Chem. Eng. J. 2020, 385, 123892.

11. Ji-Pan Yu, Li-Yong Yuan, Shuai Wang, Jian-Hui Lan, Li-Rong Zheng, Chao Xu, Jing Chen, Lin Wang, Zhi-Wei Huang, Wu-Qing Tao, Zhi-Rong Liu, Zhi-Fang Chai, John K. Gibson and Wei-Qun Shi*. Phosphonate Decorated Covalent Organic Frameworks for Actinide Extraction: a Breakthrough under Highly Acidic Conditions.

CCS Chem. 2019, 1, 286–295. (Co-first authors)

12. Xin-Rui Zhang, Xiang-He Kong, Li-Yong Yuan*, Zhi-Fang Chai, Wei-Qun Shi*. The coordination of Eu(III) with 1,10-phenanthroline-2,9-dicarboxamide derivatives: a combined study by MS, TRLIF, and DFT.

Inorg. Chem. 2019, 58, 15, 10239-10247.

13. Li-Yong Yuan, Ming Tian, Jian-Hui Lan, Xing-Zhong Cao, Xiao-Lin Wang, Zhi-Fang Chai, John K. Gibson, and Wei-Qun Shi*. Defects Engineering in Metal−Organic Frameworks: A New Strategy to Develop Applicable Actinide Sorbents.

Chem. Commun. 2018, 54, 370-373

14. Xin-Rui Zhang, Li-Yong Yuan*, Zhi-Fang Chai, Wei-Qun Shi*. Towards understanding the correlation between UO22+ extraction and substitute groups in 2,9-diamide-1,10 -phenanthroline.

Sci. China Chem. 2018, 61(10), 1285-1292.

15. Li-Yong Yuan, Lin Zhu, Cheng-Liang Xiao*, Qun-Yan Wu, Nan-Zhang, Ji-Pan Yu, Zhi-Fang Chai, Wei-Qun Shi*. Large pore 3-D cubic mesoporous (KIT-6) hybrid bearing hard-soft donor combined ligand for enhancing U(VI) capture: an experimental and theoretical investigation.

ACS Appl. Mater. Interfaces. 2017, 9 (4), 3774–3784.

16. Nan Zhang, Li-yong Yuan*, Wen-Lu Guo, Shi-Zhong Luo*, Zhi-Fang Chai, Wei-Qun Shi*. Extending the Using of Highly Porous Functionalized MOFs to Th(VI) capture.

ACS Appl. Mater. Interfaces. 2017, 9 (30), 25216–25224.

17. Lin Wang, Li-yong Yuan, Ke Chen, Yujuan Zhang, Qihuang Deng, Shiyu Du, Qing Huang*, Lirong Zheng, Jing Zhang, Zhifang Chai, Michel W. Barsoum, Xiangke Wang, Weiqun Shi*. Loading actinides in multi-layered structures for nuclear waste treatment: the first case study of uranium capture with vanadium carbide MXene.

ACS Appl. Mater. Interfaces. 2016, 8, 16396-16403. (Co-first authors)

研究队伍